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Modulation transfer spectroscopy of 7Li D1 line

Journal of Quantitative Spectroscopy and Radiative Transfer. 2025. No. 346. Article 109594.
Khalutornykh L., Saakyan S., Nazarov A., Zelener B.

We present the first implementation of modulation transfer spectroscopy (MTS) on the D1 line of 7 Li, carried
out in a compact heat-pipe vapor cell with cold windows. By varying the pump and probe intensities and
polarization configurations, we systematically map the MTS error-signal amplitude, effective linewidth, and
slope for the ground-state crossover resonance 𝐹 = 1 × 2 → 𝐹 ′ = 2. We observe Rabi-induced power broadening
and identify optimal conditions for laser frequency stabilization via tightly focused beams with total power
below 1 mW. The lin⟂lin polarization configuration yields a sharp, symmetric, high-contrast error signal with
a maximal slope. Our findings establish the MTS spectrum of the 7 Li D1 line transitions as a reliable frequency
reference for quantum technology and ultracold atom experiments, particularly in scenarios where frequency
stabilization must be achieved with low laser optical power.

Research target: Physics
Language: English
Full text
DOI
Keywords: lithiumлитийAtomic spectroscopyАтомная спектроскопияmodulation-transfer spectroscopyспектроскопия с переносом модуляции
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