• A
  • A
  • A
  • АБВ
  • АБВ
  • АБВ
  • A
  • A
  • A
  • A
  • A
Обычная версия сайта
  • RU
  • EN
  • HSE University
  • Publications
  • Articles
  • Direct measurement of ultrafast intersystem crossing time for the PtIVBr62− complex
  • RU
  • EN
Расширенный поиск
Высшая школа экономики
Национальный исследовательский университет
Priority areas
  • business informatics
  • economics
  • engineering science
  • humanitarian
  • IT and mathematics
  • law
  • management
  • mathematics
  • sociology
  • state and public administration
by year
  • 2028
  • 2027
  • 2026
  • 2025
  • 2024
  • 2023
  • 2022
  • 2021
  • 2020
  • 2019
  • 2018
  • 2017
  • 2016
  • 2015
  • 2014
  • 2013
  • 2012
  • 2011
  • 2010
  • 2009
  • 2008
  • 2007
  • 2006
  • 2005
  • 2004
  • 2003
  • 2002
  • 2001
  • 2000
  • 1999
  • 1998
  • 1997
  • 1996
  • 1995
  • 1994
  • 1993
  • 1992
  • 1991
  • 1990
  • 1989
  • 1988
  • 1987
  • 1986
  • 1985
  • 1984
  • 1983
  • 1982
  • 1981
  • 1980
  • 1979
  • 1978
  • 1977
  • 1976
  • 1975
  • 1974
  • 1973
  • 1972
  • 1971
  • 1970
  • 1969
  • 1968
  • 1967
  • 1966
  • 1965
  • 1964
  • 1963
  • 1958
  • More
Subject
News
August 25, 2026
Scientists Develop Algorithm for More Reliable Processors in Data Centres
Researchers from HSE MIEM and Samara University have developed the LRF-3D algorithm to automatically bypass idle nodes in three-dimensional networks-on-chip. Thanks to its hierarchical architecture, the algorithm outperforms existing solutions in both speed and path accuracy, improving processor reliability for use in data centres, supercomputers, and AI computing. The source code and test results are publicly available.
August 24, 2026
Researchers Develop Method for Direct Generation of Regulatory DNA
Researchers at HSE University have developed a model for generating promoters and enhancers—DNA sequences that regulate gene activity. The model works directly with DNA nucleotides, without first transforming them into a continuous numerical representation. This solution could be useful for applications in synthetic biology and gene therapy. The study results were presented at the ICLR 2026 Workshop ‘Generative AI in Genomics (Gen^2): Barriers and Frontiers.’
August 21, 2026
Social Integration: At the Crossroads of Knowledge and Values
The International Laboratory for Social Integration Research (ILSIR) at HSE University studies the challenges faced by vulnerable groups and explores ways to help them participate fully in everyday life. To develop effective solutions, the laboratory’s researchers combine cutting-edge methods with practical fieldwork. In this interview with the HSE News Service, Laboratory Head Elena Iarskaia-Smirnova discusses the laboratory’s work.

 

Have you spotted a typo?
Highlight it, click Ctrl+Enter and send us a message. Thank you for your help!

Publications
  • Books
  • Articles
  • Chapters of books
  • Working papers
  • Report a publication
  • Research at HSE

?

Direct measurement of ultrafast intersystem crossing time for the PtIVBr62− complex

Mendeleev Communications. 2020. Vol. 30. No. 4. P. 509–511.
Melnikov A., Pozdnyakov I., Chekalin S., Glebov E.

The time of ultrafast intersystem crossing for the PtIVBr62– complex in aqueous solution was measured by a fluorescence up-conversion technique. The corresponding time constant (140 ± 40 fs) is in agreement with that estimated from previous ultrafast transient absorption measurements and with the reported results of theoretical calculations.

Research target: Chemistry Physics
Language: English
Full text
DOI
Text on another site
Keywords: Ultrafast spectroscopyMetal complexes
Similar publications
Metastability of lipid vesicle shapes in uniaxial extensional flow
Pikina E., Physical Review E - Statistical, Nonlinear, and Soft Matter Physics 2026 Vol. 113 No. 5
In this work, we investigate the elastic properties of deflated vesicles and their shape dynamics in uniaxial extensional flow. By analyzing the Helfrich bending energy and viscous flow stresses in the limit of highly elongated shapes, we demonstrate that all stable vesicle configurations are metastable. For vesicles with small reduced volume, we identify the type ...
Added: September 1, 2026
HF Heating Effects as Seen From Below and Above: First Results of Joint SURA–Ionosfera-M Experiment
Chernyshov A., Padokhin A. M., Grach S. M. et al., Geophysical Research Letters 2026 Vol. 53 P. 1–11
This paper presents the first results of a coordinated experiment on the ionospheric plasma response to high-frequency (HF) overdense heating, conducted using the SURA heating facility and the Ionosfera-M satellite. The experiment combined ground-based observations with in situ satellite measurements, enabling a comprehensive study of artificial ionospheric disturbances. During the experiment, the SURA facility transmitted ...
Added: August 31, 2026
Hectometric Continuum Radiation Observations on Different Temporal Scales in Near-Earth Space
D. A. Dorofeev, A. A. Chernyshov, Mogilevsky M. M. et al., JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS 2025 Vol. 130 Article e2025JA033900
This study analyzes data from the ERG (Arase) satellite over a period of nearly 7 years (2017–2023). During this time, about 1,000 cases of hectometric continuum (HMC) radiation in near‐Earth space were detected, which made it possible to identify characteristic features on different time scales. On a daily scale, it was established that HMC is ...
Added: August 31, 2026
On the nature of hectometric continuum-type emissions in the near-Earth plasma
Mogilevsky M. M., Shaposhnikov V., Chernyshov A. et al., Physics of Plasmas 2025 Vol. 32 P. 1–10
The ERG (Arase) satellite recently discovered a non-thermal hectometric continuum with a narrowband frequency structure. The mechanism behind the generation of this type of emission in the near-Earth plasma is still unknown. This study examines the potential use of electron cyclotron harmonics instability to explain the line structure of hectometric radio emissions for the first ...
Added: August 31, 2026
(111)-Textured p-Type PbTe Films Grown on Muscovite Micawith High Room-Temperature Hole Mobility
Kobtsev Danil, Albert J., Nitzan M. et al., Applied Sciences (Switzerland) 2026 Vol. 16 No. 17 Article 8577
AIVBVI semiconductors, particularly lead chalcogenides, remain key materials for mid-wave infrared (MWIR) photodetection due to their narrow bandgap and exceptional carrier transport properties. However, the realization of high-quality p-type PbTe thin films, suitable for p–n junction devices, remains a technological challenge. In this work, we report the fabrication of high-mobility p-type PbTe thin films grown on ...
Added: August 30, 2026
Сборник трудов XXXII Международной научно-технической конференции «Радиолокация, навигация, связь»
Воронеж: Издательский дом ВГУ, 2026.
В сборник вошли материалы XXXII Международной научно-технической конференции «Радиолокация, навигация, связь» (RLNC*2026), прошедшие ре цензирование членами программного комитета конференции. Основной целью конференции является организация взаимодействия научных и научно технических коллективов для обмена опытом и новыми творческими успехами. Достижение этой цели также способствует внедрению перспективных разрабо ток, имеющих практическое значение для дальнейшего развития промышленно сти, экономики ...
Added: August 29, 2026
Pyramidal solitons: existence, instability, and interactions
Melnikov I., Pelinovsky E., Nonlinear Dynamics 2026 No. 114 Article 934
Pyramidal solitons (solitons with more than two inflection points) of the generalized Korteweg–de Vries (KdV) equation are investigated. Necessary and sufficient conditions for the existence of such structures are presented. Within the framework of the generalized Gardner equation — the simplest model that admits pyramidal solitons as solutions — it is shown that these solutions ...
Added: August 27, 2026
Non-epitaxial perovskite polariton laser diode operating under direct current
Zhukov A., Kryzhanovskaya N., Moiseev E. et al., Nature 2026 Vol. 656 P. 80–85
Reaching lasing in electrically pumped microdevices based on solution-processed semiconductors poses a substantial scientific and technological challenge. Halide perovskites offer a promising platform for electrical injection1, as their optically excited single-crystal cavities2–4 and predesigned5,6 or postprocessed microstructures7,8 have exhibited low lasing threshold. Indirect electrical pumping of a dual-cavity perovskite laser was recently obtained9, using a well-established technological concept of embedding a ...
Added: August 27, 2026
Monometallic Ln3+ and heterometallic Ln3+–Cd2+ complexes based on pentafluorophenylacetic acid: efficient control of dimension and luminescent properties
Belousov Y., Кискин М. А., Sidoruk A. et al., Australian Journal of Chemistry 2022 Vol. 75 No. 9 P. 572–580
Four new complexes [Ln(pfaa)3(H2O)2]n (Ln = Eu (1), Tb (2)) and [Ln2Cd2(pfaa)10 (phen)2(EtOH)2]·2MeCN (Ln = Eu (3), Tb (4), phen = 1,10-phenanthroline) based on pentaphorphenylacetic acid (Hpfaa) have been prepared and completely investigated. The structures of compounds 1 and 3 were studied by single crystal X-ray diffraction analysis: the isostructural complexes 1 and 2 represent ...
Added: August 26, 2026
Understanding the electric double layer at electrode–electrolyte interfaces, Part III: crystallographic-face dependence of silver capacitance in aqueous NaF solutions
Mazur D., Brandyshev P., Doronin S. V. et al., Electrochimica Acta 2026 Vol. 577 Article 149729
The electric double layer (EDL) at a single-crystal metal surface is controlled not only by the electrolyte composition and the electrode potential, but also by the atomic structure of the surface itself. This makes the Ag(hkl)/NaF interface a stringent test for continuum theories of the EDL. In the third part of our series, we examine ...
Added: August 20, 2026
Giant magnetocaloric effect in the quaternary Fe–Rh–Pd–Ir alloy: Experimental and first-principles study
Gimaev R., Karpenkov A., Shelkovyi F. et al., Journal of Alloys and Compounds 2026 No. 1080 Article 190307
The magnetothermal properties of the quaternary Fe49Rh46.1Pd3.1Ir1.8 alloy are investigated by a combination of first-principles calculations, structural characterization, magnetometry, calorimetry, and direct measurements of the adiabatic temperature change. An exceptional magnetocaloric response is obtained, with ΔTad reaching −11.9 K in a field of 1.85 T under the discontinuous protocol and −8.6 K under the continuous ...
Added: August 18, 2026
Quantum viscosity mechanism of dissipative dynamics in the Dicke model expressed via Lindblad equation of motion
Beck M. E., Seidov S., Mukhin S., Physical Review A: Atomic, Molecular, and Optical physics 2026 Vol. 113 No. 6 Article 063706
Quantum dissipation is studied in the superradiant phase of the extended Dicke model. It is demonstrated analytically by quantum mechanical derivation of the Lindblad equation for the Dicke model in the superradiant state coupled to Caldeira-Leggett thermal bath that the effective viscosity appearing in the semiclassical equations of motion of polaritonic condensate survives in the zero-temperature limit ...
Added: August 13, 2026
Analytical solution of coupled self-consistency and linearized Usadel equations for dirty superconductors near 𝑇𝑐 and with the proximity effect
S. S. Seidov, N. G. Pugach, Physical Review B: Condensed Matter and Materials Physics 2026 Vol. 114 No. 7 Article 074504
In this manuscript we consider a superconducting film in the vicinity of the critical temperature and presence of the proximity effect. We analytically solve the corresponding linearized Usadel equation and the self-consistency equation, defining the critical temperature. This is a system of coupled differential and integral equations for the anomalous Green's function and the order parameter of ...
Added: August 13, 2026
Hadrons in N = 2 supersymmetric QCD from non-Abelian string on 2D black hole
Ievlev E., Marshakov A., Sumbatian G. et al., Physical Review D - Particles, Fields, Gravitation and Cosmology 2026 Vol. 114 Article 046006
We continue the study of non-Abelian vortex string in 4D N =2 supersymmetric QCD (SQCD) as critical superstring, and extend this analysis to UðNÞ gauge theory with arbitrary even N and Nf = 2N number of quarks. We introduce a special mass deformation and show that the SQCD hadron spectrum is still given by the string spectrum on the ...
Added: August 13, 2026
Production of Λ hyperons in 4.0A GeV and 4.5A GeV carbon-nucleus interactions at the Nuclotron
Afanasiev S., Agakishiev G., Aleksandrov A. et al., Journal of High Energy Physics 2026 Vol. 2026 Article 48
The BM@N experiment (Baryonic Matter at the Nuclotron) is the first fixed-target experiment at the JINR NICA accelerator complex. In this work, data on the interactions of a carbon-ion beam with kinetic energies of 4.0A GeV and 4.5A GeV with C, Al, Cu, and Pb targets are used to measure transverse momentum spectra and rapidity ...
Added: August 12, 2026
Hall effect in electrolyte solutions: Self-consistent Debye–Hückel–Onsager theory
Budkov Y., Kalikin N., Journal of Chemical Physics 2026 Vol. 165 Article 064506
A self-consistent statistical-mechanical theory of the Hall effect in electrolyte solutions is developed by extending the self-consistent Debye–Hückel–Onsager (SCDHO) framework to crossed electric and magnetic fields. The theory incorporates non-local ionic charge distributions via Slater-type form factors, regularizing the Coulomb interaction at short range, and accounts for dielectric friction through ion-specific coefficients, employing experimental values ...
Added: August 12, 2026
Charge-controlled binding, alloy synergy, and the copper anomaly in Au–Ag–Cu dimers to clusters: DFT-derived design rules for targeted drug delivery
Novikov A., New Journal of Chemistry 2026 Vol. 50 P. 13931–13957
The rational design of coinage metal nanocarriers requires a mechanistic understanding of metal-drug binding and predictive descriptors that translate molecular interactions into design rules. Using DFT (B3LYP-D3BJ/def2-TZVP, SMD water), we systematically investigated the binding of 5-fluorouracil (5-FU) and levodopa (l-DOPA) to neutral and cationic homo- and heteronuclear dimers of Au, Ag, and Cu (Au2, Ag2, ...
Added: August 12, 2026
Ultrafast dynamics of excitons and charge carriers in Van der Waals WS2 nanotubes
Paukov M. I., Starchenko V. V., Melnikov A. et al., Materials Today Chemistry 2024 No. 36 Article 101886
Added: July 24, 2025
Selective Pathway toward Heteroleptic Spin-Crossover Iron(II) Complexes with Pyridine-Based N-Donor Ligands
Nikovskiy I., Aleshin D., Valentin V. Novikov et al., Inorganic Chemistry 2022 Vol. 61 No. 51 P. 20866–20877
A new synthetic pathway is devised to selectively produce previously elusive heteroleptic iron(II) complexes of terpyridine and N,N′-disubstituted bis(pyrazol-3-yl)pyridines that stabilize the opposite spin states of the metal ion. Such a combination of the ligands in a series of the heteroleptic complexes induces the spin-crossover (SCO) not experienced by the homoleptic complexes of these ligands or ...
Added: January 31, 2023
Synthesis of donor-π-acceptor porphyrins for DSSC: DFT-study, comparison of anchoring mode and effectiveness
Ezhov A. V., Vyal'ba F. Y., Zhdanova K. A. et al., Journal of Porphyrins and Phthalocyanines 2020 Vol. 24 No. 4 P. 538–547
n this study two pairs of novel zinc-porphyrin complexes (ZnP1 ZnP2 ZnP3 and ZnP4) were synthesized as sensitizers for DSSC and their photophysical, computational studies and photovoltaic properties were investigated. Structures of proposed dyes are based on a molecular design that relies on donor/π-bridge/acceptor interactions. Compounds differ by anchoring mode to the titanium dioxide surface: ...
Added: December 6, 2021
Formation and decay of a triplet state of dipyrido[3,2-a:2′,3′-c]phenazine
Glebov E., Bakulina O. D., Shushakov A. A. et al., Mendeleev Communications 2020 Vol. 30 No. 3 P. 322–324
The photophysical and photochemial properties of dipyrido[3,2-a:2′,3′-c]phenazine (dppz) in acetonitrile have been investigated by laser flash photolysis and ultrafast pump-probe spectroscopy. The excitation of dppz to the first singlet excited state was followed by vibrational cooling with solvent relaxation for ∼3 ps and then intersystem crossing for ∼50 ps. Spectral and kinetic characteristics of the triplet excited ...
Added: January 18, 2021
Primary processes in photochemistry of 2,3-bis(2,5-dimethylthiophen-3-yl)cyclopent-2-enone
Glebov E., Pozdnyakov I., Semionova V. V. et al., Mendeleev Communications 2020 Vol. 30 No. 1 P. 61–63
Early processes in photochemistry of 2,3-bis(2,5-dimethylthiophen-3-yl)cyclopent-2-enone were explored using the ultrafast pump-probe spectroscopy. The photocyclization occurs from the antiparallel conformation of an open form on a time scale of 7 ps, while the parallel conformation exhibits an intersystem crossing within 130 ps. The mechanism and timescales were revealed as typical of other thiophene-containing diarylethenes. ...
Added: January 18, 2021
Mechanistic study of the trans,cis,cis-[RuCl2(DMSO)2(H2O)2] complex photochemistry in aqueous solutions
Shushakov A. A., Matveeva S. G., Pozdnyakov I. et al., Photochemical and Photobiological Sciences 2020 Vol. 19 P. 1222–1229
It is known that trans,cis,cis-[RuCl2(DMSO)2(H2O)2] (1a) complexes, which are formed upon dissolution of trans-[RuCl2(DMSO)4] in water, demonstrate light-induced cytotoxicity. The mechanistic study of 1a photochemistry has been performed using ultrafast pump–probe spectroscopy, laser flash photolysis and stationary photolysis. The first stage of 1a photochemistry is the photoexchange of a DMSO ligand to a water molecule; its quantum yield is wavelength-dependent (estimating ...
Added: January 18, 2021
Photochemistry of hexachloroosmate (IV) in ethanol
Glebov E., Matveeva S. G., Pozdnyakov I. et al., Photochemical and Photobiological Sciences 2020 Vol. 19 P. 1569–1579
The photochemistry of the OsIVCl62− complex in ethanol was studied by means of stationary photolysis, nanosecond laser flash photolysis, ultrafast pump–probe spectroscopy and quantum chemistry. The direction of the photochemical process was found to be wavelength-dependent. Irradiation in the region of the d–d and LMCT bands results in the photosolvation (with the wavelength-dependent quantum yield) and ...
Added: January 18, 2021
  • About
  • About
  • Key Figures & Facts
  • Sustainability at HSE University
  • Faculties & Departments
  • International Partnerships
  • Faculty & Staff
  • HSE Buildings
  • HSE University for Persons with Disabilities
  • Public Enquiries
  • Studies
  • Admissions
  • Programme Catalogue
  • Undergraduate
  • Graduate
  • Exchange Programmes
  • Summer University
  • Summer Schools
  • Semester in Moscow
  • Business Internship
  • Research
  • International Laboratories
  • Research Centres
  • Research Projects
  • Monitoring Studies
  • Conferences & Seminars
  • Academic Jobs
  • Yasin (April) International Academic Conference on Economic and Social Development
  • Media & Resources
  • Publications by staff
  • HSE Journals
  • Publishing House
  • iq.hse.ru: commentary by HSE experts
  • Library
  • Economic & Social Data Archive
  • Video
  • HSE Repository of Socio-Economic Information
  • HSE1993–2026
  • Contacts
  • Copyright
  • Privacy Policy
  • Site Map
Edit