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Superconductivity in Cu Co-Doped SrxBi2Se3 Single Crystals
In this study, we grew Cu co-doped single crystals of a topological superconductor candidate SrxBi2Se3, and studied their structural and transport properties. We reveal that the addition of even as small an amount of Cu co-dopant as 0.6 atomic %, completely suppresses superconductivity in SrxBi2Se3. Critical temperature (∼2.7 K) is rather robust with respect to co-doping. We show that Cu systematically increases the electron density and lattice parameters a and c. Our results demonstrate that superconductivity in SrxBi2Se3-based materials is induced by significantly lower Sr doping level x<0.02 than commonly accepted x∼0.06, and it strongly depends on the specific arrangement of Sr atoms in the host matrix. The critical temperature in superconductive Sr-doped Bi2Se3 is shown to be insensitive to carrier density.