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Optical gain appearance in the CdSe/CdS nanoplatelets colloidal solution
Results in Physics. 2022. Vol. 32. Article 105120.
Alexander M. Smirnov, Golinskaya A., Mantsevich V., Kozlova M., Ezhova K., Saidzhonov B., Vasiliev R.
The experimental investigations of the colloidal heterostructured CdSe/CdS nanoplatelets transient absorption in the regime of one-photon stationary excitation of excitons by high-intensity nanosecond laser pulses are presented. A strong dependence of exciton’s transitions behavior on nanoplatelets concentration in colloidal solution and pump intensities was studied for the first time. The revealed nonlinear transmission changes of the nanoplatelets solutions with different optical density were explained by the presence of phase space filling effect, energy exchange between exciton states, reabsorption processes and exciton–exciton interaction. The most vital result of the paper is the identification of conditions for the existence of the optical gain in colloidal solutions of nanoplatelets.
Melentiev P. N., Калмыков А. С., Гритченко А. С. et al., Успехи физических наук 2024 Т. 194 № 11 С. 1130–1145
Представлен краткий обзор достигнутого уровня оптических методов детектирования единичных молекул в биомедицинских приложениях. Показано, что регистрация флуоресценции единичных молекул красителей, ковалентно связанных с антителами (биомолекулами), совместно с использованием современных методов нанофотоники может быть применена для решения различных задач в биологии и медицине: визуализации биомолекул, токсинов, вирусных частиц, определения ультранизких концентраций аналитов напрямую во взятой пробе, ...
Added: May 21, 2026
Antsiferov P.S., Stepanov L.V., Matiukhin N. D., Review of Scientific Instruments 2025 Vol. 96 No. 12 Article 123506
The article presents the discharge plasma based source of extreme ultraviolet (EUV) radiation. The discharge circuit has been driven by means of stripe line storage with working voltage 10.5 kV. The main feature of the proposed source is that plasma electrons acquire the energy, necessary for the production of multiply charged ions with ionization potentials ...
Added: May 20, 2026
Анциферов П. С., Степанов Л. В., Матюхин Н. Д., Оптика и спектроскопия 2026 Т. 134 № 2 С. 214–218
Сообщено о разработке системы регистрации спектров на ПЗС-линейке для уникального ВУФ спектрометра, построенного на основе сферической дифракционной решетки с радиусом 6.65 m. Была использована линейка HAMAMATSU S11156-2048-02, которая устанавливалась по касательной к окружности Роуланда с возможностью механического перемещения для сканирования спектра. Были получены спектрограммы в диапазоне длин волн 2130-2270 Angstrem. Описана методика сшивки регистрируемых спектральных ...
Added: May 20, 2026
Shipilov F., Barnyakov A., Ivanov A. et al., / Series Physics "arxiv.org". 2026.
A fast simulation of the detector response is a vital task in high-energy physics (HEP). Traditional Monte-Carlo methods form the backbone of modern particle physics simulation software but are computationally expensive. We present a machine-learning-based approach to fast simulation of the Focusing Aerogel Ring Imaging Cherenkov (FARICH) detector response. Given a particle track and momentum, ...
Added: May 19, 2026
Malinovsky A. M., Пилипенко С. В., Mikhalchenko A. O. et al., Astronomy Reports 2026 Vol. 70 P. 1–6
Radiation from rotational transitions of CO molecules in distant galaxies creates a chaotic background with an intensity reaching 1000 Jy/sr at a wavelength of approximately 1 mm. This background will pose a serious problem, when measuring spectral distortions of the cosmic microwave background, in particular, the mu-distortion, which presumably has an intensity of less than ...
Added: May 19, 2026
Kaveev A. K., Fedorov V. V., Pavlov A. V. et al., Journal of Materials Chemistry C 2026 Vol. 14 No. 7 P. 2697–2705
Bismuth nanostructures represent a promising material platform for semiconductor nanooptoelectronics and colorimetry owing to the multi-colored light reflection and quantum confinement. In this work, we study the photoluminescent properties of bismuth nanostructures grown using molecular beam epitaxy on the planar CaF2/Si(111) surface. We demonstrate the different surface morphologies of Bi, ranging from planar films obtained ...
Added: May 19, 2026
Pavlova T., V.M. Shevlyuga (Шевлюга В. М., Applied Surface Science 2026 Vol. 736 P. 166813–166813
The objective of miniaturizing doped areas in silicon, with the ultimate goal of achieving atomic-precision doping, requires a fundamental understanding of the dopant incorporation process at the atomic level. We present a combined scanning tunneling microscopy (STM) and density functional theory (DFT) investigation of single phosphorus atom incorporation into the Si(100) surface. Phosphorus was supplied ...
Added: May 19, 2026
Pasternak D., Romshin A., Khmelnitsky Р. et al., Carbon 2026 Vol. 256 Article 121655
A single-photon source (SPS) is a key component required for quantum communication devices. We report the
discovery of bright diamond-based SPS created by nature. It is shown that narrow (≤2 nm) lines observed in the
500-800 nm range in photoluminescence (PL) spectra of the surface layer of untreated Yakut diamonds rich in
nitrogen and hydrogen are linked to ...
Added: May 19, 2026
A.M. Smirnov, Kurtina D. A., Saitov S. R. et al., Optical Materials: X 2026 Vol. 30 Article 100441
Chiral semiconductor nanostructures and nanoparticles are promising materials for applications in biological sensing, enantioselective separation, photonics, and spin-polarized devices. Here we performed a detailed analysis of optical properties of chiral CdSe nanoplatelets with thickness of 2 and 3 monolayers (ML) with Nacetyl-L-cysteine ligands. We studied the absorption spectra peculiarities, analyzed time-resolved photoluminescence and investigated circular ...
Added: May 18, 2026
Smirnov A., Mantsevich V. N., Saitov S. R. et al., Journal of Applied Physics 2026 Vol. 139 Article 185702
This work presents a comprehensive investigation into the temperature-dependent thermally stimulated conductivity and photoconductivity of vacuum-annealed thin films based on core–shell CdSe/CdS nanoplatelets passivated with oleic acid ligands. Controlled thermal annealing under vacuum conditions leads to a substantial increase in both dark and photoinduced conductivity, which is primarily attributed to partial desorption of the ligands. ...
Added: May 18, 2026
Масютин Д. А., Moiseev E., Komarov S. et al., Письма в Журнал технической физики 2026 Т. 52 № 7 С. 27–30
Исследованы инжекционные полупроводниковые микролазеры с кольцевым резонатором радиусом 15 мкм с несимметричным расположением внутреннего отверстия резонатора. Показано, что асимметрия обеспечивает формирование в диаграмме направленности двух лепестков излучения, разориентированных на 50° относительно оси смещения внутреннего отверстия. Измеренная добротность резонаторов сопоставима с добротностью дисковых резонаторов и находится на уровне ∼ 10^6. ...
Added: May 18, 2026
Rathish S., Andrey S. Vasenko, Thazhathenair A. et al., The Journal of Physical Chemistry Letters 2026 Vol. 17 No. 18 P. 5386–5394
We demonstrate and rationalize the effect of Au nanoparticles (NPs) on the hierarchical g-C3N4/CeO2 heterojunction. g-C3N4/CeO2 decorated with monodispersed plasmonic Au NPs was synthesized. Detailed analyses showed that CeO2 nanocubes and monodispersed Au NPs were evenly distributed over the 2D g-C3N4 surface, forming a robust interface enriched with abundant active sites. The structure enabled efficient separation of photogenerated charge ...
Added: May 16, 2026
Das A., Paul R., Sharma N. et al., Colloids and Surfaces A: Physicochemical and Engineering Aspects 2026 Vol. 728 P. 138830
Niobium-doped TiO2 (Nb-TiO2), demonstrates dual functionality as an efficient photocatalyst for dye degradation and a promising photoelectrocatalyst for water oxidation. Nb incorporation via a facile hydrothermal method was confirmed by XRD (Rietveld refinement), XPS, TEM, FT-IR, Raman, and BET analyses, indicating successful lattice doping and structural modification. Photocatalytic dye degradation experiments were conducted using a model ...
Added: May 16, 2026
I. V. Kolokolov, V. V. Lebedev, Physical Review E - Statistical, Nonlinear, and Soft Matter Physics 2026 Vol. 113 No. 5 Article 054117
We theoretically investigate the correlation functions of the phase of a light wave propagating through a
turbulent medium. We use an equation for the logarithm of a wave packet envelope, which includes a secondorder
nonlinear term. Based on this equation, we develop a diagrammatic technique to calculate corrections
to the correlation function obtained in the linear approximation. We ...
Added: May 15, 2026
Гущина В. А., / Series chemrxiv-2023-vpzhz-v2 "ChemRxiv". 2023.
All-inorganic perovskite CsPbBr3 and Cs4PbBr6 nanoparticles are being intensively studied due to their unique properties and wide range of applications; however, however, the nature of their optical properties is not yet fully understood due to the difficulty of synthesis of singlephase nanoparticles. In this article we describe the features of the synthesis of single-phase particles ...
Added: May 14, 2026
Гущина В. А., Mendeleev Communications 2025 Vol. 35 No. 2 P. 193–195
All-inorganic perovskite CsPbBr3 and Cs4PbBr6 nanoparticles are intensively studied for their unique optical properties, though synthesizing single-phase nanoparticles has posed challenges. Detailed synthesis method of CsPbBr3 and Cs4PbBr6 single-phase nanoparticles and their chemical and phase analysis are described. Distinctive optical characteristics, such as photoluminescence, optical band gap and the Urbach tail region, are revealed and explained within the current ...
Added: May 14, 2026
Гущина В. А., Physics of Complex System 2026 Vol. 7 No. 1 P. 3–15
Heterostructures based on ZnO nanorods and CsPbBr3 nanocrystals were investigated for their potential as semiconductor SERS substrates. We found that ZnO morphology governs the efficiency of interfacial energy transfer, leading to enhanced photoluminescence under 390 nm excitation and a noticeable reduction of the bandgap in the composites. Raman analysis revealed a pronounced intensity enhancement and ...
Added: May 14, 2026
Fominykh N., Stegailov V., Journal of Chemical Physics 2025 Vol. 163 No. 11 Article 114704
First-principles modeling of exciton dynamics coupled with lattice vibrations is important for understanding exciton mobility, which is crucial for various applications. In order to shed light on such coupled exciton–lattice dynamics, in this paper, we use a restricted open-shell Kohn–Sham approach, which is a computationally efficient method for electronic structure calculations in the lowest excited ...
Added: September 16, 2025
Tan J., Jiang X., Liu D. et al., The Journal of Physical Chemistry Letters 2025 Vol. 16 No. 30 P. 7659–7665
Two-dimensional (2D) Ruddlesden–Popper (RP) perovskites are considered as promising optoelectronic materials due to their intriguing broadband emission properties. However, the origin of the broadband emission in RP perovskites remains a controversial issue. Herein, we have systematically analyzed the exciton behavior and luminescence properties of 2D (PEA)2PbI4. Our calculations demonstrate that 2D (PEA)2PbI4 exhibits significant quantum confinement ...
Added: July 25, 2025
Ilya D. Fedorov, Vladimir V. Stegailov, Journal of Chemical Physics 2024 Vol. 161 No. 15 Article 154503
Understanding the properties of molecular nitrogen N2 at extreme conditions is the fundamental problem for atomistic theory and the important benchmark for the capabilities of first-principles molecular dynamics (FPMD) methods. In this work, we focus on the connection between the dynamics of ions and electronic excitations in warm dense N2. The restricted open-shell Kohn–Sham method gives ...
Added: December 24, 2024
Klimenko G. A., A. Hasan, Yakimov B. P. et al., Journal of Luminescence 2024 Vol. 275 Article 120732
Peculiarities of photoluminescence (PL) and absorption spectra of gradient nanocrystals CdSe1-xSx colloidal solution were studied by pump and probe technique under stationary excitation of excitons by nanosecond laser pulses. The PL peaks and differential transmission peaks positions changing were revealed with the CdSe1-xSx nanocrystals composition variation. Bleaching of excitons transitions was observed for high pump ...
Added: June 20, 2024
Gavrilov S. Y., A. M. Smirnov, Kozlova M. V. et al., Journal of Experimental and Theoretical Physics 2023 Vol. 136 No. 5 P. 549–554
The nonlinear absorption and photoluminescence of CdTe/CdSe nanotetrapod colloids have been studied by the pump–probe method for the case of single-photon nonresonance excitation of excitons. A competition between the short-wave and long-wave shifts of the peak of photoluminescence associated with an indirect electron–hole transition, which is observed with increasing excitation radiation intensity, has been found and ...
Added: February 1, 2024