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Strong Local Field Enhancement of Raman Scattering Observed in Metal-Dielectric Gratings due to Vertical Fabry-Perot Modes of Surface Plasmon Polaritons

Physical Review Applied. 2022. Vol. 17. No. 2. Article 024015.
Gromyko D., Dyakov S., Gippius N., Weiss T., Tikhodeev S., Astrakhantseva A., Yana V. Fedotova, Kukushkin I.

The height dependence of Raman light scattering on organic molecules deposited onto thick onedimensional metal-dielectric gratings is investigated theoretically and experimentally. We observe oscillations of the intensity of Raman light scattering as a function of the height of the metastructure’s strips and demonstrate that these oscillations are explicitly associated with a type of Fabry-Perot effect. We show that the intensity of surface-enhanced Raman scattering can be additionally increased by local field enhancement (by an order of magnitude) at resonances of both pump and Stokes as well as anti-Stokes frequency, due to coupling of the surface plasmon polaritons on the top and bottom metal parts of the gratings via the vertical Fabry-Perot resonances over their middle dielectric part. A semianalytical one-mode model to describe the effect qualitatively is proposed. A significant deviation of the dispersion of Fabry-Perot-coupled plasmon polaritons from the surface-plasmon-polariton dispersion just folded into the first Brillouin zone is demonstrated.

Research target: Physics
Language: English
Full text
DOI
Keywords: nanoplasmonics and nanophotonics
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