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June 5, 2026
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Chiral excitations and the intermediate-field regime in the Kitaev magnet 𝛼−RuCl3

Physical Review Research. 2024. Vol. 6. No. 2. Article L022005.
Sahasrabudhe A., Mikhail A. Prosnikov, Koethe T., Stein P., Tsurkan V., Loidl A., Grüninger M., Hedayat H., van Loosdrecht P. .

In the Kitaev magnet 𝛼⁢-RuCl3, the existence of a magnetic-field-induced quantum spin-liquid phase and of anyonic excitations is controversially discussed. We address this elusive, exotic phase via helicity-dependent Raman scattering and analyze the Raman optical activity of excitations as a function of magnetic field and temperature. The hotly debated field regime between 7.5 and 10.5T is characterized by clear spectroscopic signatures such as a plateau of the Raman optical activity of the dominant, chiral spin-flip excitation. This provides direct evidence for the existence of a distinct intermediate-field regime with an intriguing ground state featuring chiral excitations

Research target: Physics
Language: English
DOI
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Keywords: magnetismquantum phase transitionshigh magnetic fields Raman spectroscopy
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